FEL2015 - List of Keywords (scattering)

Paper	Title	Other Keywords	Page
MOP085	Scheme to Increase the Output Average Spectral Flux of the European XFEL at 14.4 keV	FEL, undulator, electron, photon	251
	V. Kocharyan, E. Saldin DESY, Hamburg, Germany G. Geloni XFEL. EU, Hamburg, Germany
	Inelastic X-ray scattering and nuclear resonance scattering are limited by the photon flux available at SR sources, up to 10¹⁰ ph/s/meV at 14.4 keV. A thousand-fold increase may be obtained by exploiting high repetition rate self-seeded pulses at the European XFEL. We report on a feasibility study for an optimized configuration of the SASE2 beamline combining self-seeding and undulator tapering at 14.4 keV. One should perform monochromatization at 7.2 keV by self-seeding, and amplify the seed in the first part of the output undulator. Before saturation, the electron beam is considerably bunched at the 2nd harmonic. A second part of the output undulator tuned to 14.4 keV can thus be used to obtain saturation at this energy. One can further prolong the exchange of energy between the photon and the electron beam by tapering the last part of the output undulator. Start-to-end simulations demonstrate that self-seeding, combined with undulator tapering, allows one to achieve more than a hundred-fold increase in average spectral flux compared with the nominal SASE regime at saturation, resulting in a spectral flux of order 10¹³ ph/s/meV. A more detailed description of this study can be found in. G. Geloni, V. Kocharyan and E.~Saldin, "Scheme to increase the output average spectral flux of the European XFEL at 14.4 keV", DESY 15-141 (2015).
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MOP086	Novel Opportunities for Sub-meV Inelastic X-Ray Scattering Experiments at High-Repetition Rate Self-seeded XFELs	undulator, radiation, photon, optics	257
	O.V. Chubar BNL, Upton, Long Island, New York, USA G. Geloni, A. Madsen XFEL. EU, Hamburg, Germany V. Kocharyan, E. Saldin, S. Serkez DESY, Hamburg, Germany Yu. Shvyd'ko ANL, Argonne, Ilinois, USA J. Sutter DLS, Oxfordshire, United Kingdom
	Inelastic x-ray scattering (IXS) is an important tool for studies of equilibrium dynamics in condensed matter. A new spectrometer recently proposed for ultra-high-resolution IXS (UHRIX) has achieved 0.6 meV and 0.25/nm spectral and momentum Transfer resolutions, respectively. However, further improvements down to 0.1 meV and 0.02/nm are required to close the gap in energy-momentum space between high and low frequency probes. We Show that this goal can be achieved by further improvements in x-ray optics and by increasing the spectral flux of the incident x-ray pulses. UHRIX performs best at energies from 5 to 10 keV, where a combination of self-seeding and undulator tapering at the SASE2 beamline of the European XFEL promises up to a hundred-fold increase in average spectral flux compared to nominal SASE pulses at saturation, or three orders of magnitude more than possible with storage-ring based radiation sources. Wave-optics propagation shows that about 7·10¹² ph/s in a 90-microeV bandwidth can be achieved on the sample. This will provide unique new possibilities for IXS. Extended information about our work can be found in. Y. Shvyd'ko et al., Nature Communications 5:4219 (2014). ** O. Chubar et al., ‘Novel opportunities for sub-meV inelastic X-ray scattering at high-repetition rate self-seeded X-ray free-electron lasers', http://arxiv.org/abs/1508.02632, DESY 15-140, (2015).
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TUP009	Coherent Thomson Scattering Using the PEHG	radiation, laser, electron, simulation	351
	S. Chen, K. Ohmi, D. Zhou KEK, Ibaraki, Japan
	Electron beam is density modulated by the phase-merging effect to obtain ultra-short longitudinal structures in the phase space. Coherent radiations are then generated by the coherent Thomson scattering between the phase-merged beam and a long wavelength laser pulse.
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WEP010	Development of Phonon Dynamics Measurement System by MIR-FEL and Pico-second Laser	FEL, laser, timing, lattice	615
	T. Murata, T. Katsurayama, T. Kii, T. Konstantin, K. Masuda, T. Nogi, H. Ohgaki, S. Suphakul, K. Torgasin, H. Zen Kyoto University, Kyoto, Japan K. Hachiya Kyoto University Graduate School of Energy Science, Kyoto, Japan K. Yoshida Kumamoto University, Department of Applied Chemistry and Biochemistry, Kumamoto, Japan
	Coherent control of a lattice vibration in bulk solid (mode-selective phonon excitation: MSPE) is one of the attractive methods in the solid state physics because it becomes a powerful tool for the study of ultrafast lattice dynamics (e.g. electron-phonon interaction and phonon-phonon interaction). Not only for that, MSPE can control electronic, magnetic, and structural phases of materials. In 2013, we have directly demonstrated MSPE of a bulk material with MIR-FEL (KU-FEL) by anti-Stokes Raman scattering spectroscopy. For the next step, we are starting a phonon dynamics measurement to investigate the difference of physical property between thermally excited phonon (phonon of equilibrium state) and optically excited phonon (phonon of non-equilibrium state) by time-resolved method in combination with a pico-second VIS laser. By using pico-second laser, we also expect to perform the anti-Stokes hyper-Raman scattering spectroscopy to extend MSPE method to the phonon mode which has Raman inactive . As the first step, we have commissioned the time-resolved phonon measurement system and started measurement on 6H-SiC. In this conference, we will present the outline of measurement system, and experimental results.
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Paper

Title

Other Keywords

Page

MOP085

Scheme to Increase the Output Average Spectral Flux of the European XFEL at 14.4 keV

FEL, undulator, electron, photon

251

V. Kocharyan, E. Saldin
DESY, Hamburg, Germany
G. Geloni
XFEL. EU, Hamburg, Germany

Inelastic X-ray scattering and nuclear resonance scattering are limited by the photon flux available at SR sources, up to 10¹⁰ ph/s/meV at 14.4 keV. A thousand-fold increase may be obtained by exploiting high repetition rate self-seeded pulses at the European XFEL. We report on a feasibility study for an optimized configuration of the SASE2 beamline combining self-seeding and undulator tapering at 14.4 keV. One should perform monochromatization at 7.2 keV by self-seeding, and amplify the seed in the first part of the output undulator. Before saturation, the electron beam is considerably bunched at the 2nd harmonic. A second part of the output undulator tuned to 14.4 keV can thus be used to obtain saturation at this energy. One can further prolong the exchange of energy between the photon and the electron beam by tapering the last part of the output undulator. Start-to-end simulations demonstrate that self-seeding, combined with undulator tapering, allows one to achieve more than a hundred-fold increase in average spectral flux compared with the nominal SASE regime at saturation, resulting in a spectral flux of order 10¹³ ph/s/meV. A more detailed description of this study can be found in*.
* G. Geloni, V. Kocharyan and E.~Saldin, "Scheme to increase the output average spectral flux of the European XFEL at 14.4 keV", DESY 15-141 (2015).

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MOP086

Novel Opportunities for Sub-meV Inelastic X-Ray Scattering Experiments at High-Repetition Rate Self-seeded XFELs

undulator, radiation, photon, optics

257

O.V. Chubar
BNL, Upton, Long Island, New York, USA
G. Geloni, A. Madsen
XFEL. EU, Hamburg, Germany
V. Kocharyan, E. Saldin, S. Serkez
DESY, Hamburg, Germany
Yu. Shvyd'ko
ANL, Argonne, Ilinois, USA
J. Sutter
DLS, Oxfordshire, United Kingdom

Inelastic x-ray scattering (IXS) is an important tool for studies of equilibrium dynamics in condensed matter. A new spectrometer recently proposed for ultra-high-resolution IXS (UHRIX) has achieved 0.6 meV and 0.25/nm spectral and momentum Transfer resolutions, respectively*. However, further improvements down to 0.1 meV and 0.02/nm are required to close the gap in energy-momentum space between high and low frequency probes. We Show that this goal can be achieved by further improvements in x-ray optics and by increasing the spectral flux of the incident x-ray pulses. UHRIX performs best at energies from 5 to 10 keV, where a combination of self-seeding and undulator tapering at the SASE2 beamline of the European XFEL promises up to a hundred-fold increase in average spectral flux compared to nominal SASE pulses at saturation, or three orders of magnitude more than possible with storage-ring based radiation sources. Wave-optics propagation shows that about 7·10¹² ph/s in a 90-microeV bandwidth can be achieved on the sample. This will provide unique new possibilities for IXS. Extended information about our work can be found in**.
* Y. Shvyd'ko et al., Nature Communications 5:4219 (2014).
** O. Chubar et al., ‘Novel opportunities for sub-meV inelastic X-ray scattering at high-repetition rate self-seeded X-ray free-electron lasers', http://arxiv.org/abs/1508.02632, DESY 15-140, (2015).

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TUP009

Coherent Thomson Scattering Using the PEHG

radiation, laser, electron, simulation

351

S. Chen, K. Ohmi, D. Zhou
KEK, Ibaraki, Japan

Electron beam is density modulated by the phase-merging effect to obtain ultra-short longitudinal structures in the phase space. Coherent radiations are then generated by the coherent Thomson scattering between the phase-merged beam and a long wavelength laser pulse.

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reference for this paper to ※ LaTeX, ※ Text, ※ IS/RefMan, ※ EndNote (xml)

WEP010

Development of Phonon Dynamics Measurement System by MIR-FEL and Pico-second Laser

FEL, laser, timing, lattice

615

T. Murata, T. Katsurayama, T. Kii, T. Konstantin, K. Masuda, T. Nogi, H. Ohgaki, S. Suphakul, K. Torgasin, H. Zen
Kyoto University, Kyoto, Japan
K. Hachiya
Kyoto University Graduate School of Energy Science, Kyoto, Japan
K. Yoshida
Kumamoto University, Department of Applied Chemistry and Biochemistry, Kumamoto, Japan

Coherent control of a lattice vibration in bulk solid (mode-selective phonon excitation: MSPE) is one of the attractive methods in the solid state physics because it becomes a powerful tool for the study of ultrafast lattice dynamics (e.g. electron-phonon interaction and phonon-phonon interaction). Not only for that, MSPE can control electronic, magnetic, and structural phases of materials. In 2013, we have directly demonstrated MSPE of a bulk material with MIR-FEL (KU-FEL) by anti-Stokes Raman scattering spectroscopy. For the next step, we are starting a phonon dynamics measurement to investigate the difference of physical property between thermally excited phonon (phonon of equilibrium state) and optically excited phonon (phonon of non-equilibrium state) by time-resolved method in combination with a pico-second VIS laser. By using pico-second laser, we also expect to perform the anti-Stokes hyper-Raman scattering spectroscopy to extend MSPE method to the phonon mode which has Raman inactive . As the first step, we have commissioned the time-resolved phonon measurement system and started measurement on 6H-SiC. In this conference, we will present the outline of measurement system, and experimental results.

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reference for this paper to ※ LaTeX, ※ Text, ※ IS/RefMan, ※ EndNote (xml)