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Liang, J. F.

Paper Title Page
FPAE053 Isobar Suppression by Photodetachment in a Gas-Filled RF Quadrupole Ion Guide 3250
 
  • Y. Liu, J.R. Beene, C.C. Havener, J. F. Liang
    ORNL, Oak Ridge, Tennessee
  • A.C. Havener
    University of Tennessee, Knoxville, Tennessee
  
  Funding: Managed by UT-Battelle, LLC, for the U.S. DOE under contract DE-AC05-00OR22725. Co-author Aaron Havener was under a U.S. DOE Science Undergraduate Laboratory Internship.

A novel method is described for selective suppression of isobar contaminants in negative radioactive ion beams. Negative ion beams extracted from an ion source were decelerated to low energies and injected into a gas-filled radio-frequency quadrupole (RFQ) ion guide where the ions were cooled and unwanted ions were selectively removed by non-resonant photodetachment with photons of sufficient energy. Simulation studies show that the laser-ion interaction time in a 40 cm long RFQ ion guide can be on the order of milliseconds, thus, high efficiency photodetachment is possible with commercially available CW lasers. There are a number of adjacent-Z species whose negative ions are such that photodetachment can be used to suppress the unwanted negative ion species while leaving the species of interest intact. Examples of particular interest include suppressing the 56Co- component in a mixed 56Ni- + 56Co- beam and the 17O- component in a mixed 17O- + 17F- beam. In a proof–of-principle experiment a CW Nd:YAG laser at 1064 nm wavelength was used to selectively remove Co- ions in the (Ni, Co) pair. With laser power on the order of 3 W, 95% of Co- beams were suppressed while only 10% of Ni- beams were neutralized in a He-filled RFQ guide.