Taran Driver (SLAC National Accelerator Laboratory)
TUAI1
Cascaded Amplification of Attosecond X-Ray Pulses: Towards TW-Scale Ultrafast X-Ray Free-Electron Lasers
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The natural time scale of valence electronic motion in molecular systems is on the order of hundreds of attoseconds. Consequently, the time-resolved study of electronic dynamics requires a source of sub-femtosecond pulses. Pulses in the soft x-ray domain can access core-level electrons, enabling the study of site-specific electron dynamics through attosecond pump/probe experiments. As time-resolved pump/probe experiments are nonlinear processes, these experiments require high brightness attosecond x-ray pulses. The X-ray Laser-Enhanced Attosecond Pulses (XLEAP) collaboration is an ongoing project for the development of attosecond x-ray modes at the Linac Coherent Light Source (LCLS). Here we report development of a high power attosecond mode via cascaded amplification of the x-ray pulse. We experimentally demonstrate generation of sub-femtosecond duration soft x-ray free electron laser pulses with hundreds of microjoules of energy. In conjunction with the upcoming high repetition rate at LCLS-II, these tunable, high intensity attosecond capabilities enable new nonlinear spectroscopic techniques and advanced imaging methods. This work was supported by US Department of Energy Contracts No. DE-AC02-76SF00 and the Basic Energy Sciences Accelerator and Detector Research Program.
Paper: TUAI1
DOI: reference for this paper: 10.18429/JACoW-FEL2022-TUAI1
About: Received: 17 Aug 2022 — Revised: 25 Aug 2022 — Accepted: 25 Aug 2022 — Issue date: 13 Jul 2023